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Polypyrrole PPy nanocomposites incorporating different carbon nanostructures CNS , including graphenes of different sizes, carbon nanofibers CNFs and carbon nanotubes CNTs , have been successfully synthesized using a surface initiated polymerization SIP method. The effects of graphene size, loading level and surface functionality on the electrical conductivity and dielectric permittivity of their corresponding nanocomposites have been systematically studied. The electron transportation mechanism has been investigated, which follows a quasi 3-d variable range hopping VRH behavior in the nanocomposites. Scanning electron microscopy and transmission electron microscopy results indicate that the PPy coating on one-dimensional carbon nanostructures , such as CNFs and CNTs, is more smooth and uniform than that on the two-dimensional graphenes.

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